Preparation and Catalytic Performance of Gold Nanoparticles Supported on Periodic Mesoporous Organosilica of SBA-15

Chinese Journal of Catalysis ›› 2009, Vol. 30 ›› Issue (9): 896-900.

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Preparation and Catalytic Performance of Gold Nanoparticles Supported on Periodic Mesoporous Organosilica of SBA-15

ZHUANG Daying1, JIN Yong1,2, YU Ningya1,*, QIN Liangsheng2, LIU Jianfu2, YIN Donghong1,2,#, YANG Cuiqing2

1Institute of Fine Catalysis and Synthesis, Key Lab of Sustainable Resources Processing and Advanced Materials of Hunan Province,Hunan Normal University, Changsha 410081, Hunan, China 2Technology Center, China Tobacco Hunan Industrial Corporation, Changsha 410014, Hunan, China

Received:2009-09-25 Online:2009-09-25 Published:2009-09-25

Abstract

Abstract: Gold nanoparticles in the channels of disulfide functionalized periodic mesoporous organosilica were used as the catalyst for the selective oxidation of benzyl alcohol by aqueous t-butyl hydroperoxide (TBHP). A benzyl alcohol conversion of 29.1% with 100% selectivity for benzaldehyde was achieved, and the catalyst could be conveniently recovered and recycled.

Key words: gold nanoparticle, functionalized periodic mesoporous organosilica, ionic liquid, benzyl alcohol, benzyaldehyde

ZHUANG Daying;JIN Yong;YU Ningya;*;QIN Liangsheng;LIU Jianfu;YIN Donghong;#;YANG Cuiqing. Preparation and Catalytic Performance of Gold Nanoparticles Supported on Periodic Mesoporous Organosilica of SBA-15[J]. Chinese Journal of Catalysis, 2009, 30(9): 896-900.

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Preparation and Catalytic Performance of Gold Nanoparticles Supported on Periodic Mesoporous Organosilica of SBA-15

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