H2 Production with Low CO Selectivity from Photocatalytic Reforming of Glucose on Ni/TiO2-SiO2

doi:10.1016/S1872-2067(10)60276-8

Abstract

Abstract: Nano-sized Ni particles on TiO₂-SiO₂ were synthesized by the two methods of photo-assisted deposition (PAD) and impregnation. H₂, which is a promising energy carrier, with a low CO concentration was produced by the photocatalytic reforming of glucose (a model biomass) on the Ni/TiO₂-SiO₂ catalyst. The supported Ni enhanced the rate of H₂ production while it suppressed CO selectivity. The catalysts were characterized by X-ray diffraction, X-ray absorption fine structure, transmission electron microscope, and nitrogen adsorption analysis. Both H₂ production and CO selectivity were strongly dependent on the preparation method, and PAD-Ni/TiO₂-SiO₂ was the better catalyst for H₂ production with the lowest CO concentration.

Key words: titanium dioxide, silicon dioxide, nickel doping, hydrogen production

R. M. MOHAMED, Elham S. AAZAM. H₂ Production with Low CO Selectivity from Photocatalytic Reforming of Glucose on Ni/TiO₂-SiO₂[J]. Chinese Journal of Catalysis, 2012, 33(2): 247-253.

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H₂ Production with Low CO Selectivity from Photocatalytic Reforming of Glucose on Ni/TiO₂-SiO₂

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