The role of alkali promoters in enhancing the direct N2O decomposition reactivity over NiO catalysts

doi:10.1016/S1872-2067(15)60963-9

Abstract

Abstract:

Direct N₂O decomposition has been investigated over bare NiO and a series of its alkali-promoted catalysts. These catalysts were characterized by X-ray diffractometry, X-ray photoelectron spectroscopy (XPS) and field emission scanning electron microscopy. XPS analysis revealed that surface nickel is present in three forms: metal particles, NiO and Ni(OH)₂. It is suggested that nickel(0) valent atoms are essential for the interaction with N₂O molecules at the catalyst surfaces. Bare NiO exhibited a very low N₂O decomposition reactivity. However, the alkali-containing catalysts exhibited a marked activity enhancement.

Key words: N₂O decomposition, Greenhouse gas, NiO, Alkali-promotion, Activity enhancement

Bahaa M. Abu-Zied, Abdullah M. Asiri. The role of alkali promoters in enhancing the direct N₂O decomposition reactivity over NiO catalysts[J]. Chinese Journal of Catalysis, 2015, 36(11): 1837-1845.

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URL: https://www.cjcatal.com/EN/10.1016/S1872-2067(15)60963-9

https://www.cjcatal.com/EN/Y2015/V36/I11/1837

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The role of alkali promoters in enhancing the direct N₂O decomposition reactivity over NiO catalysts

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