Pt/Bi24O31Cl10 composite nanosheets with significantly enhanced photocatalytic activity under visible light irradiation

doi:10.1016/S1872-2067(18)63156-0

Abstract

Abstract:

Efficient composite semiconductor photocatalysts are highly desirable for the visible-light-driven degradation of organic pollutants. In this study, Bi₂₄O₃₁Cl₁₀ photocatalyst was prepared via a hydrothermal method and modified with Pt nanoparticles (NPs) through a facile deposition procedure. The composite photocatalyst was characterized by X-ray diffraction, transmission electronic microscopy, X-ray photoelectron spectroscopy, UV-vis diffusion reflectance spectroscopy, photoluminescence spectroscopy, and electron spin resonance. The 1.0 wt% Pt/Bi₂₄O₃₁Cl₁₀ photocatalyst showed the highest activity for the degradation of methyl orange under visible light (source:300 W Xe lamp coupled with a UV-cutoff filter), and the photocatalytic degradation efficiency improved about 2.2 times compared to that of pure Bi₂₄O₃₁Cl₁₀. The composite photocatalyst could maintain most of its activity after four runs of the photocatalytic experimental cycle. This study could provide a novel insight for the modification of other desirable semiconductor materials to achieve high photocatalytic activities.

Key words: Bismuth-based oxyhalide, Photocatalyst, Bi₂₄O₃₁Cl₁₀, Methyl orange degradation

Boran Xu, Juan Li, Lu Liu, Yandong Li, Shaohui Guo, Yangqin Gao, Ning Li, Lei Ge. Pt/Bi₂₄O₃₁Cl₁₀ composite nanosheets with significantly enhanced photocatalytic activity under visible light irradiation[J]. Chinese Journal of Catalysis, 2019, 40(5): 713-721.

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URL: https://www.cjcatal.com/EN/10.1016/S1872-2067(18)63156-0

https://www.cjcatal.com/EN/Y2019/V40/I5/713

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Pt/Bi₂₄O₃₁Cl₁₀ composite nanosheets with significantly enhanced photocatalytic activity under visible light irradiation

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