Facet-dependent anchoring of gold nanoparticles on TiO2 for CO oxidation

doi:10.1016/S1872-2067(19)63388-7

Abstract

Abstract: The interfacial perimeter of gold nanocatalysts is popularly viewed as the active sites for a number of chemical reactions, while the geometrical structure of the interface at atomic scale is less known. Here, TiO₂-nanosheets and nanospindles were adapted to accommodate Au particles (~2.2 nm), forming Au-TiO₂{001} and Au-TiO₂{101} interfaces. Upon calcination at 623 K in air, HAADF-STEM images evidenced that the Au particles on TiO₂{101} enlarged to 3.1 nm and these on TiO₂{001} remained unchanged, suggesting the stronger metal-support interaction on TiO₂{001}. Au/TiO₂{001} was more active for CO oxidation than Au/TiO₂{101} system.

Key words: Au nanoparticles, Titanium dioxide, Stability, Interfacial perimeter, CO oxidation

Bin Shao, Wenning Zhao, Shu Miao, Jiahui Huang, Lili Wang, Gao Li, Wenjie Shen. Facet-dependent anchoring of gold nanoparticles on TiO₂ for CO oxidation[J]. Chinese Journal of Catalysis, 2019, 40(10): 1534-1539.

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Facet-dependent anchoring of gold nanoparticles on TiO₂ for CO oxidation

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