The crystalline linear polyimide with oriented photogenerated electron delivery powering CO2 reduction

doi:10.1016/S1872-2067(23)64xxx-x

Abstract

Abstract: Orienting electron transport to suppress charge recombination is attractive for efficient photocatalysis but remains challenging. Herein, we demonstrate the synthesis of crystalline linear conjugated polyimides via the condensation of carboxylic anhydrides and amine monomers for the photocatalytic reduction of CO₂. Oriented electron transport was achieved using crystalline polyimides integrated with electronic push-pull units. Directional intramolecular electron transfer is driven by the dipole effects of the adjacent building units. The sulfone-based polyimide exhibited excellent photocatalytic performance for CO₂ reduction. Our work provides a new example photoreduction of CO₂ and a strategy for developing efficient photocatalysts with oriented electron transport.

Key words: Photocatalysis, Crystalline polymer, Polyimides, CO₂ reduction, Electron transport

Huizhen Li, Yanlei Chen, Qing Niu, Xiaofeng Wang, Zheyuan Liu, Jinhong Bi, Yan Yu, Liuyi Li. The crystalline linear polyimide with oriented photogenerated electron delivery powering CO₂ reduction[J]. Chinese Journal of Catalysis, DOI: 10.1016/S1872-2067(23)64xxx-x.

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The crystalline linear polyimide with oriented photogenerated electron delivery powering CO₂ reduction

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