Synthesis of H2O2 and High-Value Chemicals by COF-based Photocatalysts

Abstract

Abstract: Hydrogen peroxide (H₂O₂) is a versatile and environmentally friendly oxidizer widely used in diverse fields. The solar-driven photocatalytic oxygen reduction reaction (ORR) generates H₂O₂ from air and water, avoiding undesirable by-products. This green and pollution-free route is applicable across various domains. While existing research extensively covers covalent organic framework (COF) based photocatalysts for H₂O₂, little attention is given to systems generating high-value chemicals with scavengers. To address this gap, we systematically discuss photocatalysis generating H₂O₂ and valuable chemicals, simultaneously. We emphasize pathways for H₂O₂ generation using COF-based photocatalysts, highlighting the role of sacrificial agents. Novel synthetic methodologies and modification strategies to enhance photocatalytic yield are presented. Our contribution extends to identifying and discussing challenges faced by photocatalysts in this area. This work aims to inspire further investigations and innovations in COF-based photocatalysis for sustainable and value-added chemical synthesis by presenting a holistic view.

Gaoxiong Liu, Rundong Chen, Bingquan Xia, Zhen Wu, Shantang Liu, Jingrun Ran. Synthesis of H₂O₂ and High-Value Chemicals by COF-based Photocatalysts[J]. Chinese Journal of Catalysis.

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Synthesis of H₂O₂ and High-Value Chemicals by COF-based Photocatalysts

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