光催化还原 CO2 的研究现状和发展前景

doi:10.3724/SP.J.1088.2011.10509

摘要/Abstract

摘要： 综述了光催化还原 CO2 的研究进展, 并重点介绍了本课题组在光催化还原 CO2 为碳氢燃料方面的研究工作, 通过该途径可降低 CO2 在大气中的排放浓度, 还可将 CO2 转化为烷烃、醇或其它有机物质, 从而实现碳材料的再循环使用. 最后展望了该研究领域的前景.

关键词: 光催化, 二氧化碳, 还原, 碳氢化合物

Abstract: CO₂ photoreduction as typical advanced technology has been becoming one of the most promising solutions to mitigate CO₂ emissions. Firstly, emission reduction and utilization of CO₂ was introduced. Then the present research status of photocatalytic conversion of CO₂ was reviewed, with particular attention to our recent progress on this field. The artificial photosynthesis technology helps one partially reduce atmospheric CO₂ levels and fulfill the recycle utilization of CO₂. Finally, challenges and prospects for further development of this field are presented.

Key words: photocatalysis, carbon dioxide, reduction, hydrocarbons

吴聪萍, 周勇, 邹志刚. 光催化还原 CO₂ 的研究现状和发展前景[J]. 催化学报, 2011, 32(10): 1565-1572.

WU Cong-Ping, ZHOU Yong, ZOU Zhi-Gang. Research Progress in Photocatalytic Conversion of CO₂ to Hydrocarbons[J]. Chinese Journal of Catalysis, 2011, 32(10): 1565-1572.

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参考文献

1Singh D, Croiset E, Douglas P L, Douglas M A. Energy Converse Manage, 2003, 44: 3073
2Rao A B, Rubin E S. Environ Sci Technol, 2002, 36: 4467
3White C M, Strazisar B R, Granite E J, Hoffman J S, Pennline H W. J Air Waste Manage Assoc, 2003, 53: 645
4Voormeij D A, Simandl G J. Geosci Canada, 2004, 31: 11
5Indrakanti V P, Kubicki J D, Schobert H H. Energy Envir Sci, 2009, 2: 745
6Roy S C, Varghese O K, Paulose M, Grimes C A. ACS Nano, 2010, 4: 1259
7Palmisano G, García-López E, MarcíG, Loddo V, Yurdakal S, Augugliaro V, Palmisano L. Chem Commun, 2010, 46: 7074
8Hoffmann M R, Moss J A, Baum M M. Dalton Trans, 2011, 40: 5151
9Halmann M. Nature, 1978, 275: 115
10Inoue T, Fujishima A, Konishi S, Honda K. Nature, 1979, 277: 637
11Halmann M, Ulman M, Aurian-Blajeni B. Solar Energy, 1983, 31: 429
12Anpo M, Yamashita H, Ichihashi Y, Fujii Y, Honda M. J Phys Chem B, 1997, 101: 2632
13Ikeue K, Yamashita H, Anpo M, Takewaki T. J Phys Chem B, 2001, 105: 8350
14Ikeue K, Nozaki S, Ogawa M, Anpo M. Catal Today, 2002, 74: 241
15Yamashita H, Ikeue K, Takewaki T, Anpo M. Top Catal, 2002, 18: 95
16Dimitrijevic N M, Vijayan B K, Poluektov O G, Rajh T, Gray K A, He H, Zapol P. J Am Chem Soc, 2011, 133: 3964
17Ishitani O, Inoue H, Suzuki Y, Ibusuki T. J Photochem Photobiol A, 1993, 72: 269
18Tseng I H, Wu J C S, Chou H Y. J Catal, 2004, 221: 432
19Liu B J, Torimoto T, Matsumoto H, Yoneyama H. J Photochem Photobiol A, 1997, 108: 187
20Varghese O K, Paulose M, LaTempa T J, Grimes C A. Nano Lett, 2009, 9: 731
21Wang C, Thompson R L, Baltrus J, Matranga C. J Phys Chem Lett, 2010, 1: 48
22Woolerton T W, Sheard S, Reisner E, Pierce E, Ragsdale S W, Armstrong F A. J Am Chem Soc, 2010, 132: 2132
23徐用军, 周定, 姜琳琳, 李向久, 刘崇微, 刘金尧. 哈尔滨工业大学学报 (Xu Y J, Zhou D, Jiang L L, Li X J, Liu Ch W, Liu J Y. J Harbin Inst Technol), 2000, 32: 104
24陈崧哲, 钟顺和, 肖秀芬. 催化学报 (Chen S Zh, Zhong Sh H, Xiao X F. Chin J Catal), 2003, 24: 67
25赵春, 钟顺和. 应用化学 ( Zhao Ch, Zhong Sh H. Chin J Appl Chem), 2005, 22: 349
26Liu Y Y, Huang B B, Dai Y, Zhang X Y, Qin X Y, Jiang M H, Whangbo M H. Catal Commun, 2009, 11: 210
27Yang C C, Yu Y H, van der Linden B, Wu J C S, Mul G. J Am Chem Soc, 2010, 132: 8398
28Zhao Z H, Fan J M, Wang Z Z. J Clean Prod, 2007, 15: 1894
29Zhao Z H, Fan J M, Xie M M, Wang Z Z. J Clean Prod, 2009, 17: 1025
30Ozcan O, Yukruk F, Akkaya E U, Uner A D. Appl Catal B, 2007, 71: 291
31Nguyen T V, Wu J C S, Chiou C H. Catal Commun, 2008, 9: 2073
32Cao L, Sahu S, Anilkumar P, Bunker C E, Xu J, Shiral Fernando K A, Wang P, Guliants E A, Tackett K N, Sun Y P. J Am Chem Soc, 2011, 133: 4754
33Zou Z, Ye J H, Sayama K, Arakawa H. Nature, 2001, 414: 625
34Vijayakumar K M, Lichtin N N. J Catal, 1984, 90: 173
35Matsumoto Y, Obata M, Hombo J. J Phys Chem, 1994, 98: 2950
36Pan P W, Chen Y W. Catal Commun, 2007, 8: 1546
37Nguyen T V, Wu J C S. Appl Catal A, 2008, 335: 112
38Xi G C, Ouyang S X, Ye J H. Chem Eur J, 2011, 17: 9057
39Liu Q, Zhou Y, Kou J H, Chen X Y, Tian Z P, Gao J, Yan S C, Zou Z G. J Am Chem Soc, 2010, 132: 14385
40Yan S C, Wan L J, Li Z S, Zou Z G. Chem Commun, 2011, 47: 5632
41Gao F, Chen X Y, Yin K B, Dong S, Ren Z F, Yuan F, Yu T, Zou Z G, Liu J M. Adv Mater, 2007, 19: 2889
42Lü J, Kako T, Li Z S, Zou Z G, Ye J H. J Phys Chem C, 2010, 114: 6157
43Kou J H, Gao J, Li Z S, Zou Z G. Curr Org Chem, 2010, 14: 728
44Fan X X, Gao J, Wang Y, Li Z S, Zou Z G. J Mater Chem, 2010, 20: 2865
45Lü J, Kako T, Zou Z G, Ye J H. J Mater Res, 2010, 25: 159
46Lü J, Kako T, Zou Z G, Ye J H. Appl Phys Lett, 2009, 95: 032107
47Kudo A, Hijii S. Chem Lett, 1999: 1103
48Tang J W, Zou Z G, Ye J H. Catal Lett, 2004, 92: 53
49Liu Y Y, Huang B B, Dai Y, Zhang X Y, Qin X Y, Jiang M H, Whangbo M H. Catal Commun, 2009, 11: 210
50Zou X D, Conradsson T, Klingstedt M, Dadachov M S, O’Keeffe M. Nature, 2005, 437: 716
51Zhou Y, Zhu H, Chen Z, Chen M, Xu Y, Zhang H, Zhao D. Angew Chem, Int Ed, 2001, 40: 2166
52Liu G, Zheng S, Yang G. Angew Chem, Int Ed, 2007, 46: 2827
53Lin Z E, Yang G Y. Eur J Inorg Chem, 2010, 19: 2895 and the references therein
54Sato J, Kobayashi H, Ikarashi K, Saito N, Nishiyama H, Inoue Y. J Phys Chem B, 2004, 108: 4369
55Huang J H, Cui Y J, Wang X C. Environ Sci Technol, 2010, 44: 3500
56Ma B J, Wen F Y, Jiang H F, Yang J H, Ying P L, Li C. Catal Lett, 2010, 134: 78
57Xia Y N, Yang P D, Sun Y G, Wu Y Y, Mayers B, Gates B, Yin Y D, Kim F, Yan Y Q. Adv Mater, 2003, 15: 353
58Kim S S, Park J Y, Kim H S, Na H G, Yang J C, Shim S H, Lee C, Park D, Nam D, Cheong H, Kim H W. J Phys D, 2011, 44: 025502
59Li L, Lee P S, Yan C, Zhai T, Fang X, Liao M, Koide Y, Bando Y, Golberg D. Adv Mater, 2010, 22: 5145
60Su Y, Li S, Xu L, Chen Y Q, Zhou Q T, Peng B, Yin S, Meng X, Liang X M, Feng Y. Nanotechnology, 2006, 17: 6007
61Yan C, Zhang T, Lee P S. Cryst Growth Des, 2008, 8: 3144
62Zhan J H, Bando Y, Hu J Q, Yin L W, Yuan X L, Sekiguchi T, Golberg D. Angew Chem, Int Ed, 2006, 45: 228
63Yan C, Singh N, Lee P S. Cryst Growth Des, 2009, 9: 3697
64Yan C, Lee P S. J Phys Chem C, 2009, 113: 14135
65Li C, Bando Y, Liao M Y, Koide Y, Golberg D. Appl Phys Lett, 2010, 97: 161102
66Yan C, Singh N, Lee P S. Appl Phys Lett, 2010, 96: 053108
67Tsai M Y, Yu C Y, Wang C C, Perng T P. Cryst Growth Des, 2008, 8: 2264
68Huang J H, Ding K N, Hou Y D, Wang X C, Fu X Z. Chem-SusChem, 2008, 1: 1011
69Huang J H, Wang X C, Hou Y D, Chen X F, Wu L, Fu X Z. Environ Sci Technol, 2008, 42: 7387
70Song R Q, Xu A W, Yu S H. J Am Chem Soc, 2007, 129: 4152
71Wan Y, Zhao D Y. Chem Rev, 2007, 107: 2821
72Yan S C, Ouyang S X, Gao J, Yang M, Feng J Y, Fan X X, Wan L J, Li Z S, Ye J H, Zhou Y, Zou Z G. Angew Chem, Int Ed, 2010, 49: 6400
73Pichon A. Energy materials: A stretch to save the world. http://www.nature.com/nchina/2010/101103/full/nchina.2010.126.html

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光催化还原 CO₂ 的研究现状和发展前景

Research Progress in Photocatalytic Conversion of CO₂ to Hydrocarbons

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