Size dependence of photocatalytic oxidation reactions of Rh nanoparticles dispersed on (Ga1-xZnx)(N1-xOx) support

doi:10.1016/S1872-2067(14)60181-9

催化学报 ›› 2014, Vol. 35 ›› Issue (12): 1944-1954.DOI: 10.1016/S1872-2067(14)60181-9

Size dependence of photocatalytic oxidation reactions of Rh nanoparticles dispersed on (Ga_1-xZn_x)(N_1-xO_x) support

Yi Zhang, D. A. J. Michel Ligthart, Peng Liu, Lu Gao, Tiny M. W. G. M. Verhoeven, Emiel J. M. Hensen

Department of Chemical Engineering and Chemistry, Eindhoven University of Technology, P.O. Box 513, 5600 MB, Eindhoven, The Netherlands

收稿日期:2014-05-15 修回日期:2014-06-26 出版日期:2014-11-29 发布日期:2014-11-29
通讯作者: Emiel J. M. Hensen

Size dependence of photocatalytic oxidation reactions of Rh nanoparticles dispersed on (Ga_1-xZn_x)(N_1-xO_x) support

Yi Zhang, D. A. J. Michel Ligthart, Peng Liu, Lu Gao, Tiny M. W. G. M. Verhoeven, Emiel J. M. Hensen

Department of Chemical Engineering and Chemistry, Eindhoven University of Technology, P.O. Box 513, 5600 MB, Eindhoven, The Netherlands

Received:2014-05-15 Revised:2014-06-26 Online:2014-11-29 Published:2014-11-29

摘要/Abstract

摘要：

Mixed Ga-Zn oxynitrides were synthesized using coprecipitation, wet-precipitation, and solid-solution methods. The oxynitrides were used as supports for Rh nanoparticle catalysts in photocatalytic water splitting, CO oxidation, and H₂ oxidation. Mixed Ga-Zn oxynitrides produced by wet precipitation and nitridation had good visible-light-absorption properties and high surface areas, so they were used to support uniformly sized poly(vinylpyrrolidone)-stabilized Rh nanoparticles. The nanoparticle size range was 2-9 nm. These catalysts had negligible activity in photocatalytic H₂ production by water splitting with methanol as a sacrificial agent. Other mixed Ga-Zn oxynitrides were also inactive. A reference sample provided by Domen also showed very low activity. The influence of particle size on Rh-catalyzed oxidation of CO and H₂ was investigated. For CO oxidation, the activities of small particles were higher for particles with higher Rh oxidation degrees. The opposite holds for H₂ oxidation.

关键词: Oxynitride, Rhodium nanoparticle, Water splitting, Carbon monoxide oxidation, Hydrogen oxidation

Abstract:

Key words: Oxynitride, Rhodium nanoparticle, Water splitting, Carbon monoxide oxidation, Hydrogen oxidation

Yi Zhang, D. A. J. Michel Ligthart, Peng Liu, Lu Gao, Tiny M. W. G. M. Verhoeven, Emiel J. M. Hensen. Size dependence of photocatalytic oxidation reactions of Rh nanoparticles dispersed on (Ga_1-xZn_x)(N_1-xO_x) support[J]. 催化学报, 2014, 35(12): 1944-1954.

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参考文献

[1] Maeda K, Takata T, Hara M, Saito N, Inoue Y, Koboyashi H, Domen K. J Am Chem Soc, 2005, 127: 8286
[2] Maeda K, Teramura K, Takata T, Hara M, Saito N, Toda K, Inoue Y, Kobayashi H, Domen K. J Phys Chem B, 2005, 109: 20504
[3] Maeda K, Teramura K, Lu D L, Takata T, Saito N, Inoue Y, Domen K. Nature, 2006, 440: 295
[4] Yashima M, Maeda K, Teramura K, Takata T, Domen K. Chem Phys Lett, 2005, 416: 225
[5] Yashima M, Maeda K, Teramura K, Takata T, Domen K. Mater Trans, 2006, 47: 295
[6] Sun X J, Maeda K, Le Faucheur M, Teramura K, Domen K. Appl Catal A, 2007, 327: 114
[7] Hirai T, Maeda K, Yoshida M, Kubota J, Ikeda S, Matsumura M, Domen K. J Phys Chem C, 2007, 111: 18853
[8] Maeda K, Teramura K, Domen K. J Catal, 2008, 254: 198
[9] Hisatomi T, Maeda K, Lu D L, Domen K. ChemSusChem, 2009, 2: 336
[10] Hisatomi T, Miyazaki K, Takanabe K, Maeda K, Kubota J, Sakata Y, Domen K. Chem Phys Lett, 2010, 486: 144
[11] Meada K, Hashiguchi H, Masuda H, Abe R, Domen K. J Phys Chem C, 2008, 112: 3447
[12] Boppana V B R, Doren D J, Lobo R F. J Mater Chem, 2010, 20: 9787
[13] Zou L, Xiang X, Wei M, Li F, Evans D G. Inorg Chem, 2008, 47: 1361
[14] Moriya Y, Takata T, Domen K. Coord Chem Rev, 2013, 257: 1957
[15] Adeli B, Taghipour F. ECS J Solid State Sci Technol, 2013, 2: Q118
[16] Han W Q, Liu Z X, Yu H G. Appl Phys Lett, 2010, 96: 183112
[17] Lee K, Tienes B M, Wilker M B, Schnitzenbaumer K J, Dukovic G. Nano Lett, 2012, 12: 3268
[18] Ward M J, Han W Q, Sham T K. J Phys Chem C, 2013, 117: 20332
[19] Li X H, Shao C L, Wang D, Zhang X, Zhang P, Liu Y C. Ceram Int, 2014, 40: 3425
[20] Li F, Duan X. Struct Bond, 2006, 119: 193
[21] Wang J P, Huang B B, Wang Z Y, Wang P, Cheng H F, Zheng Z X, Qin X Y, Zhang X Y, Dai Y, Whangbo M H. J Mater Chem, 2011, 21: 4562
[22] Mapa M, Thushara K S, Saha B, Chakraborty P, Janet C M, Viswanath R P, Nair C M, Murty K V G K, Gopinath C S. Chem Mater, 2009, 21: 2973
[23] Maeda K, Sakamoto N, Ikeda T, Ohtsuka H, Xiong A K, Lu D L, Kanehara M, Teranishi T, Domen K. Chem Eur J, 2010, 16: 7750
[24] Ikeda T, Xiong A K, Yoshinaga T, Maeda K, Domen K, Teranishi T. J Phys Chem C, 2013, 117: 2467
[25] Ligthart D A J M, van Santen R A, Hensen E J M. Angew Chem Int Ed, 2011, 50: 5306
[26] Ligthart D A J M, van Santen R A, Hensen E J M. J Catal, 2011, 280: 206
[27] Zhang Y, Ligthart D A J M, Quek X Y, Gao L, Hensen E J M. Int J Hydrogen Energy, 2014, 39: 11537
[28] Grass M E, Zhang Y W, Butcher D R, Park J Y, Li Y M, Bluhm H, Bratlie K M, Zhang T F, Somorjai G A. Angew Chem Int Ed, 2008, 47: 8893
[29] Aliaga C, Park J Y, Yamada Y, Lee H S, Tsung C K, Yang P D, Somorjai G A. J Phys Chem C, 2009, 113: 6150
[30] Yoshida M, Takanabe K, Maeda K, Ishikawa A, Kubota J, Sakata Y, Ikezawa Y, Domen K. J Phys Chem C, 2009, 113: 10151
[31] Sakamoto N, Ohtsuka H, Ikeda T, Maeda K, Lu D L, Kanehara M, Teramura K, Teranishi T, Domen K. Nanoscale, 2009, 1: 106
[32] Maeda K, Teramura K, Lu D L, Saito N, Inoue Y, Domen K. Angew Chem Int Ed, 2006, 45: 7806
[33] Maeda K, Teramura K, Lu D L, Saito N, Inoue Y, Domen K. J Phys Chem C, 2007, 111: 7554
[34] Coey J M D. Acta Crystallogr Sect B, 1970, 26: 1876
[35] Quek X Y, Guan Y J, Hensen E J M. Catal Today, 2012, 183: 72
[36] Crespo-Quesada M, Andanson J M, Yarulin A, Lim B, Xia Y N, Kiwi-Minsker L. Langmuir, 2011, 27: 7909
[37] Maeda K, Lu D L, Teramura K, Domen K. Energy Environ Sci, 2010, 3: 471
[38] Maeda K, Teramura K, Lu D L, Takata T, Saito N, Inoue Y, Domen K. J Phys Chem B, 2006, 110: 13753
[39] Kandiel T A, Dillet R, Robben L, Bahnemann D W. Catal Today, 2011, 161: 196
[40] Li Y X, Lu G X, Li S B. J Photochem Photobiol A, 2002, 152: 219
[41] Maeda K. personal communication
[42] Hahn C, Fardy M A, Nguyen C, Natera-Comte M, Andrews S C, Yang P D. Israel J Chem, 2012, 52: 1111
[43] Busser G W, Mei B, Muhler M. ChemSusChem, 2012, 5: 2200
[44] Dionigi F, Vesborg P C K, Pedersen T, Hansen O, Dahl S, Xiong A K, Maeda K, Domen K, Chorkendorff I. J Catal, 2012, 292: 26
[45] Song W Y, Jansen A P J, Degirmenci V, Ligthart D A J M, Hensen E J M. Chem Commun, 2013, 49: 3851
[46] Grass M E, Joo S H, Zhang Y W, Somorjai G A. J Phys Chem C, 2009, 113: 8616
[47] Joo S H, Park J Y, Renzas J R, Butcher D R, Huang W Y, Somorjai G A. Nano Lett, 2010, 10: 2709
[48] Park J Y, Aliaga C, Renzas J R, Lee H, Somorjai G A. Catal Lett, 2009, 129: 1
[49] Shimura K, Kawai H, Yoshida T, Yoshida H. Chem Commun, 2011, 47: 8958
[50] Shimura K, Kawai H, Yoshida T, Yoshida H. ACS Catal, 2012, 2: 2126
[51] Nilekar A U, Alayoglu S, Eichhorn B, Mavrikakis M. J Am Soc Chem, 2010, 132: 7418

Size dependence of photocatalytic oxidation reactions of Rh nanoparticles dispersed on (Ga_1-xZn_x)(N_1-xO_x) support

Size dependence of photocatalytic oxidation reactions of Rh nanoparticles dispersed on (Ga_1-xZn_x)(N_1-xO_x) support

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