近常压光电子能谱在催化领域中的应用

摘要/Abstract

摘要： 为满足催化等研究的需求，光电子能谱技术在近几十年内不断发展并开始打破真空环境中静态研究的限制，向实际催化环境中的原位动态测试方向发展。得益于同步辐射光源的迅猛发展，基于同步辐射大科学平台的近常光电子能谱（APXPS）实验站被广泛应用于能源、环境和材料领域的相关研究.本文将简要总结APXPS原位表征技术在催化领域中的应用与发展趋势.对比国内外发展现状，提出未来的发展建议.

关键词: 近常压光电子能谱, 同步辐射, 催化, 气/固界面, 液/固界面

Abstract: To bridge the "pressure gap" in catalytic research, continuous efforts have been made over the past several decades towards achieving photoelectron spectroscopy measurements at elevated pressures. With the help of bright synchrotron light sources, the ambient-pressure X-ray photoelectron spectroscopy (APXPS) endstation based on synchrotron radiation facility is widely used in researches on energy, environment and materials. Here, we will briefly summarize the application and development of in-situ APXPS characterization technique in the field of catalysis. Also, we will give our perspective on the development of APXPS in the future.

Key words: ambient-pressure X-ray photoelectron spectroscopy, synchrotron radiation, catalysis, gas/solid interface, liquid/solid interface

韩永, 章辉, 刘志. 近常压光电子能谱在催化领域中的应用[J]. 催化学报, 2019, 40(s1): 200-208.

HAN Yong, ZHANG Hui, LIU Zhi. Ambient-Pressure X-ray Photoelectron Spectroscopy in Catalysis[J]. Chinese Journal of Catalysis, 2019, 40(s1): 200-208.

×
扫码分享

导出引用管理器 EndNote|Ris|BibTeX

链接本文: https://www.cjcatal.com/CN/

https://www.cjcatal.com/CN/Y2019/V40/Is1/200

参考文献

1 Yang W L, Liu Z. In:Fan C H, Zhao Z T ed. Synchrotron Radiation in Materials Science:Light Sources, Techniques, and Applications, Wiley, 2018.511
2 Somorjai A G, Li Y M. Introduction to Surface Chemistry and Catalysis. 2nd Ed. Wiley, 2010
3 Siegbahn H, Siegbahn K. J Electron Spectroscopy Related Phenomena, 1973, 2:319
4 Siegbahn H. J Phys Chem, 1985, 89:897
5 Frank Ogletree D, Bluhm H, Lebedev G, Fadley C S, Hussain Z, Salmeron M. Rev Sci Instr, 2002, 73:3872
6 Ogletree D F, Bluhm H, Hebenstreit E D, Salmeron M. Nuclear Instr Methods Phys Res A, 2009, 601:151
7 Grass M E, Karlsson P G, Aksoy F, Lundqvist M, Wannberg B, Mun B S, Hussain Z, Liu Z. Rev Sci Instr, 2010, 81:053106
8 Starr D E, Liu Z, Havecker M, Knop-Gericke A, Bluhm H. Chem Soc Rev, 2013, 42:5833
9 Salmeron M, Schlögl R. Surf Sci Rep, 2008, 63:169
10 Arble C, Jia M, Newberg J T. Surf Sci Rep, 2018, 73:37
11 Bluhm H, Haevecker M, Knop-Gericke A, Kiskinova M, Schlöegl R, Salmeron M. MRS Bull, 2007, 32:1022
12 Salmeron M. Top Catal, 2018, 61:2044
13 Roy K, Artiglia L, van Bokhoven J A. ChemCatChem, 2018, 10:666
14 Grass M E, Zhang Y W, Butcher D R, Park J Y, Li Y M, Bluhm H, Bratlie K M, Zhang T F, Somorjai G A. Angew Chem Int Ed, 2008, 47:8893
15 Tao F, Grass M E, Zhang Y W, Butcher D R, Renzas J R, Liu Z, Chung J Y, Mun B S, Salmeron M, Somorjai G A. Science, 2008, 322:932
16 Somorjai G A, Frei H, Park J Y. J Am Chem Soc, 2009, 131:16589
17 Somorjai G A, Aliaga C. Langmuir, 2010, 26:16190
18 Tao F, Dag S, Wang L W, Liu Z, Butcher D R, Bluhm H, Salmeron M, Somorjai G A. Science, 2010, 327:850
19 Tao F, Grass M E, Zhang Y W, Butcher D R, Aksoy F, Aloni S, Altoe V, Alayoglu S, Renzas J R, Tsung C K, Zhu Z W, Liu Z, Salmeron M, Somorjai G A. J Am Chem Soc, 2010, 132:8697
20 Alayoglu S, Beaumont S K, Zheng F, Pushkarev V V, Zheng H M, Iablokov V, Liu Z, Guo J H, Kruse N, Somorjai G A. Top Catal, 2011, 54:, 778
21 Alayoglu S, Tao F, Altoe V, Specht C, Zhu Z W, Aksoy F, Butcher D R, Renzas R J, Liu Z, Somorjai G A. Catal Lett, 2011, 141:633
22 Butcher D R, Grass M E, Zeng Z H, Aksoy F, Bluhm H, Li W X, Mun B S, Somorjai G A, Liu Z. J Am Chem Soc, 2011, 133:20319
23 Alayoglu S, Krier J M, Michalak W D, Zhu Z W, Gross E, Somorjai G A. ACS Catal, 2012, 2:2250
24 Pushkarev V V, Zhu Z W, An K J, Hervier A, Somorjai G A. Top Catal, 2012, 55:1257
25 Qadir K, Joo S H, Mun B S, Butcher D R, Renzas J R, Aksoy F, Liu Z, Somorjai G A, Park J Y. Nano Lett, 2012, 12:5761
26 Zheng F, Alayoglu S, Pushkarev V V, Beaumont S K, Specht C, Aksoy F, Liu Z, Guo J H, Somorjai G A. Catal Today, 2012, 182:54
27 Zhu Z W, Tao F, Zheng F, Chang, R, Li Y M, Heinke L, Liu Z, Salmeron M, Somorjai G A. Nano Lett, 2012, 12:1491
28 Alayoglu S, Beaumont S K, Melaet G, Lindeman A E, Musselwhite N, Brooks C J, Marcus M A, Guo J G, Liu Z, Kruse N, Somorjai G A. J Phys Chem C, 2013, 117:21803
29 An K, Alayoglu S, Musselwhite N, Plamthottam S, Melaet G, Lindeman A E, Somorjai G A. J Am Chem Soc, 2013, 135:16689
30 Beaumont S K, Alayoglu S, Pushkarev V V, Liu Z, Kruse N, Somorjai G A. Faraday Dis, 2013, 162:31
31 Butcher D R, Zhu Z W, Mao B H, Wang H L, Liu Z, Salmeron M, Somorjai G A. Chem Commun, 2013, 49:6903
32 Musselwhite N, Alayoglu S, Melaet G, Pushkarev V V, Lindeman A E, An K, Somorjai G A. Catal Lett, 2013, 143:907
33 Wang H L, Krier J M, Zhu Z W, Melaet G, Wang Y H, Kennedy G, Alayoglu S, An K, Somorjai G A. ACS Catal, 2013, 3:2371
34 Wang H L, Wang Y H, Zhu Z W, Sapi A, An K, Kennedy G, Michalak W D, Somorjai G A. Nano Lett, 2013, 13:2976
35 Zhu Z W, Butcher D R, Mao B H, Liu Z, Salmeron M, Somorjai G A. J Phys Chem C, 2013, 117:2799
36 Zhu Z W, Melaet G, Axnanda S, Alayoglu S, Liu Z, Salmeron M, Somorjai G A. J Am Chem Soc, 2013, 135:12560
37 An K, Zhang Q, Alayoglu S, Musselwhite N, Shin J Y, Somorjai G A. Nano Lett, 2014, 14:4907
38 Axnanda S, Zhu Z W, Zhou W P, Mao B H, Chang R, Rani S, Crumlin E J, Somorjai, G A, Liu Z, J Phys Chem C, 2014, 118:1935
39 Michalak W D, Krier J M, Alayoglu S, Shin J Y, An K, Komvopoulos K, Liu Z, Somorjai G A. J Catal, 2014, 312:17
40 Zhu Z W, Barroo C, Lichtenstein L, Eren B, Wu C H, Mao B H, De Bocarme T V, Liu Z, Kruse N, Salmeron M, Somorjai G A. J Phys Chem Lett, 2014, 5:2626
41 Alayoglu S, Somorjai G A. Catal Lett, 2015, 145:249
42 Carenco S, Wu C H, Shavorskiy A, Alayoglu S, Somorjai G A, Bluhm H, Salmeron M. Small, 2015, 11:3045
43 Han H L, Melaet G, Alayoglu S, Somorjai G A. ChemCatChem, 2015, 7:3625
44 Alayoglu S, Somorjai G A, Top Catal, 2016, 59:420
45 Kennedy G, Melaet G, Han H L, Ralston W T, Somorjai G A. ACS Catal, 2016, 6:7140
46 Liu W C, Melaet G, Ralston W T, Alayoglu S, Horowitz Y, Ye R, Hurlburt T, Mao B H, Crumlin E J, Salmeron M, Somorjai G A. Catal Lett, 2016, 146:1574
47 Ye R, Hurlburt T J, Sabyrov K, Alayoglu S, Somorjai G A. Proc Natl Acad Sci USA, 2016, 113:5159
48 Hurlburt T J, Liu W C, Ye R, Somorjai G A. Top Catal, 2018, 61:1210
49 Ye R, Liu W C, Han H L, Somorjai G A. ChemCatChem, 2018, 10:1666
50 Miller D, Sanchez Casalongue H, Bluhm H, Ogasawara H, Nilsson A, Kaya S. J Am Chem Soc, 2014, 136:6340
51 Ketteler G, Yamamoto S, Bluhm H, Andersson K, Starr D E, Ogletree D F, Ogasawara H, Nilsson A, Salmeron M. J Phys Chem C, 2007, 111:8278
52 Andersson K, Ketteler G, Bluhm H, Yamamoto S, Ogasawara H, Pettersson L G M, Salmeron M, Nilsson A. J Am Chem Soc, 2008, 130:2793
53 Deng X, Verdaguer A, Herranz T, Weis C, Bluhm H, Salmeron M. Langmuir, 2008, 24:9474
54 Yamamoto S, Bluhm H, Andersson K, Ketteler G, Ogasawara H, Salmeron M, Nilsson A. J Phys Condensed Matter, 2008, 20:184025
55 Jiang P, Porsgaard S, Borondics F, Koeber M, Caballero A, Bluhm H, Besenbacher F, Salmeron M. J Am Chem Soc, 2010, 132:2858
56 Eren B, Heine C, Bluhm H, Somorjai G A, Salmeron M. J Am Chem Soc, 2015, 137:11186
57 Eren B, Lichtenstein L, Wu C H, Bluhm H, Somorjai G A, Salmeron M. J Phys Chem C, 2015, 119:14669
58 Eren B, Weatherup R S, Liakakos N, Somorjai G A, Salmeron M. J Am Chem Soc, 2016, 138:8207
59 Eren B, Zherebetskyy D, Hao Y, Patera L L, Wang L W, Somorjai G A, Salmeron M. Surf Sci, 2016, 651:210
60 Eren B, Zherebetskyy D, Patera L L, Wu C H, Bluhm H, Africh C, Wang L W, Somorjai G A, Salmeron M. Science, 2016, 351:475
61 Heine C, Eren B, Lechner B A J, Salmeron M. Surf Sci, 2016, 652:51
62 Heine C, Lechner B A J, Bluhm H, Salmeron M. J Am Chem Soc, 2016, 138:13246
63 Wu C H, Eren B, Bluhm H, Salmeron M. ACS Catal, 2017, 7:1150
64 Eren B, Kersell H, Weatherup R S, Heine C, Crumlin E J, Friend C M, Salmeron M. J Phys Chem B, 2018, 122:548
65 Wu C H, Liu C, Su D, Xin H L, Fang H T, Erens B, Zhang S, Murray C B, Salmeron M. Nat Catal, 2019, 2:78
66 Hua Q, Cao T, Gu X K, Lu J Q, Jiang Z Q, Pan X R, Luo L F, Li W X, Huang W X. Angew Chem Int Ed, 2014, 53:4856
67 Greiner M T, Jones T E, Klyushin A, Knop-Gericke A, Schlögl R. J Am Chem Soc, 2017, 139:11825
68 Graciani J, Mudiyanselage K, Xu F, Baber A E, Evans J, Senanayake S D, Stacchiola D J, Liu P, Hrbek J, Sanz J F, Rodriguez J A. Science, 2014, 345:546
69 Jiao F, Li J J, Pan X L, Xiao J P, Li H B, Ma H, Wei M M, Pan Y, Zhou Z Y, Li M R, Miao S, Li J, Zhu Y F, Xiao D, He T, Yang J H, Qi F, Fu Q, Bao X H. Science, 2016, 351:1065
70 Cheng K, Gu B, Liu X L, Kang J C, Zhang Q H, Wang Y. Angew Chem Int Ed, 2016, 55:4725
71 Zhu Y F, Pan X L, Jiao F, Li J, Yang J H, Ding, M, Z, Han Y, Liu Z, Bao X H. ACS Catal, 2017, 7:2800
72 Gao P, Li S G, Bu X N, Dang S S, Liu Z Y, Wang H, Zhong L S, Qiu M H, Yang C G, Cai J, Wei W, Sun Y H. Nat Chem, 2017, 9:1019
73 Axnanda S, Crumlin E J, Mao B H, Rani S, Chang R, Karlsson P G, Edwards M O M, Lundqvist M, Moberg R, Ross P N, Hussain Z, Liu Z. Sci Rep, 2015, 5:9788
74 Favaro M, Jeong B, Ross P N, Yano J, Hussain Z, Liu Z, Crumlin E J. Nat Commun, 2016, 7:12695
75 Lichterman M F, Hu S, Richter M H, Crumlin E J, Axnanda S, Favaro M, Drisdell W, Hussain Z, Mayer T, Brunschwig B S, Lewis N S, Liu Z, Lewerenz H J. Energy Environ Sci, 2015, 8:2409
76 Favaro M, Valero-Vidal C, Eichhorn J, Toma F M; Ross P N, Yano J, Liu Z, Crumlin E J. J Mater Chem A, 2017, 5:11634
77 Favaro M, Yang J, Nappini S, Magnano E, Toma F M, Crumlin E J, Yano J, Sharp I D. J Am Chem Soc, 2017, 139:8960
78 Han Y, Axnanda S, Crumlin E J, Chang R, Mao B H, Hussain Z, Ross P N, Li Y M Liu Z. J Phys Chem B, 2018, 122:666
79 Ali-Loytty H, Louie M W, Singh M R, Li L, Sanchez Casalongue H G, Ogasawara H, Crumlin E J, Liu Z, Bell A T, Nilsson A, Friebel D. J Phys Chem C, 2016, 120:2247
80 Mom R, Frevel L, Velasco-Vélez J-J, Plodinec M, Knop-Gericke A, Schlögl R. J Am Chem Soc, 2019, 141:6537
81 Cai J, Dong Q, Han Y, Mao B H, Zhang H, Karlsson P G, Åhlund J, Tai R Z, Yu Y, Liu Z. Nuclear Sci Tech, 2019, 30:81
82 Ning Y X, Fu Q, Li Y F, Zhao S Q, Wang C, Breitschaft M, Hagen S, Schaff O, Bao X H. Ultramicroscopy, 2019, 200:105

[1]	赵彬彬, 钟威, 陈峰, 王苹, 别传彪, 余火根. 高晶化g-C₃N₄光催化剂: 合成、结构调控和光催化产氢[J]. 催化学报, 2023, 52(9): 127-143.
[2]	唐小龙, 李锋, 李方, 江燕斌, 余长林. 单原子催化剂在光催化和电催化合成过氧化氢中的研究进展[J]. 催化学报, 2023, 52(9): 79-98.
[3]	张季, 俞爱民, 孙成华. 非金属掺杂石墨烯异核双原子催化剂氮还原特性研究[J]. 催化学报, 2023, 52(9): 263-270.
[4]	胡金念, 田玲婵, 王海燕, 孟洋, 梁锦霞, 朱纯, 李隽. MXene负载3d金属单原子高效氮还原电催化剂的理论筛选[J]. 催化学报, 2023, 52(9): 252-262.
[5]	洪岩, 王琦, 阚子旺, 张禹烁, 郭晶, 李思琦, 刘松, 李斌. 电化学氮还原氨反应催化剂的最新研究进展[J]. 催化学报, 2023, 52(9): 50-78.
[6]	孙嘉辰, 陈赛, 付东龙, 王伟, 王显辉, 孙国栋, 裴春雷, 赵志坚, 巩金龙. 氧扩散与表面反应在VO_x-Ce_1‒_xZr_xO₂催化丙烷脱氢反应中的影响[J]. 催化学报, 2023, 52(9): 217-227.
[7]	蔡铭洁, 刘艳萍, 董珂欣, 陈晓波, 李世杰. 漂浮型Bi₂WO₆/C₃N₄/碳布S型异质结光催化材料用于高效净化水体环境[J]. 催化学报, 2023, 52(9): 239-251.
[8]	刘勇, 赵晓丽, 隆昶, 王晓艳, 邓邦为, 李康璐, 孙艳娟, 董帆. 原位构筑动态Cu/Ce(OH)_x界面用于高活性、高选择性和高稳定性硝酸盐还原合成氨[J]. 催化学报, 2023, 52(9): 196-206.
[9]	高晖, 张恭, 程东方, 王永涛, 赵静, 李晓芝, 杜晓伟, 赵志坚, 王拓, 张鹏, 巩金龙. 构建Cu台阶位促进电催化CO₂还原制醇类化学品的研究[J]. 催化学报, 2023, 52(9): 187-195.
[10]	王思恺, 闵祥婷, 乔波涛, 颜宁, 张涛. 单原子催化: 追寻催化领域的“圣杯”[J]. 催化学报, 2023, 52(9): 1-13.
[11]	江梓聪, 程蓓, 张留洋, 张振翼, 别传彪. 氧化锌基梯型异质结光催化剂[J]. 催化学报, 2023, 52(9): 32-49.
[12]	邹心仪, 顾均. 酸性条件下二氧化碳高效电还原策略[J]. 催化学报, 2023, 52(9): 14-31.
[13]	Abhishek R. Varma, Bhushan S. Shrirame, Sunil K. Maity, Deepti Agrawal, Naglis Malys, Leonardo Rios-Solis, Gopalakrishnan Kumar, Vinod Kumar. C4二醇的发酵生产及其化学催化升级为高价值化学品的研究进展[J]. 催化学报, 2023, 52(9): 99-126.
[14]	刘鑫, 王茂弟, 任亦起, 刘嘉立, 戴慧聪, 杨启华. 构建模块化催化体系用于氢转移反应: 氢键的促进作用[J]. 催化学报, 2023, 52(9): 207-216.
[15]	赵磊, 张震, 朱昭昭, 李平波, 蒋金霞, 杨婷婷, 熊佩, 安旭光, 牛晓滨, 齐学强, 陈俊松, 吴睿. 缺陷氮掺杂碳耦合Co-N₅单原子位点用于高效锌-空气电池[J]. 催化学报, 2023, 51(8): 216-224.